Herbertsmithite Quantum Spin Liquid

  1. Identification of strongly correlated spin liquid in herbertsmithite.
  2. Quantum spin liquid observed in physics first - Cosmos.
  3. A New State Of Matter: Quantum Spin Liquids Explained.
  4. Symmetry Reduction in the Quantum Kagome Antiferromagnet Herbertsmithite.
  5. Gapless triangular-lattice spin-liquid candidate in PrZnAl$_{11}$O$_{19}.
  6. Heat Transport in Herbertsmithite: Can a Quantum Spin Liquid.
  7. Li doped kagome spin liquid compounds - The College of.
  8. For Newly Discovered 'Quantum Spin Liquid', the Beauty Is in.
  9. Quantum Spin-Liquid Behavior in the Spin-1/2 Random-Bond Heisenberg.
  10. (PDF) Quantum Spin Liquid Pathway | George Rajna - A.
  11. Fractionalized excitations in the spin-liquid state of a.
  12. Evidence for a gapped spin-liquid ground state in a kagome... - AAAS.
  13. MIT demonstrates new magnetic state with quantum spin liquids.
  14. Perfect Kagomé lattices in YCu3(OH)6Cl3: a new candidate for the.

Identification of strongly correlated spin liquid in herbertsmithite.

The apparent simplicity of Herbertsmithite belies the complexity of the spin liquid state that it apparently supports, Broholm says, which could make it useful someday. "The structural simplicity of Herbertsmithite is valuable if we are to put the quantum spin liquid to use—as proposed for information processing, for example," he says. One favorable situation for spins to enter the long-sought quantum spin liquid (QSL) state is when they sit on a kagome lattice. No consensus has been reached in theory regarding the true ground state of this promising platform. The experimental efforts, relying mostly on one archetypal material ZnCu 3 (OH) 6 Cl 2, have also led to diverse possibilities. The theoretical possibility of a "quantum spin liquid," for which there is no breaking of spin rotational symmetry, remained an intriguing possibility(5).In1973PhilipAndersonproposed that the ground state of a simple quantum mechanical model—the spin-½ antiferromag-netic near-neighborHeisenbergmodel (6)on atriangularlattice.

Quantum spin liquid observed in physics first - Cosmos.

Specific Gravity:3.85 - 3.95. Named in honor of George Frederick Herbert Smith (26 May 1872, Edgbaston, England, UK - 20 April 1953), crystallographer and curator, British Museum of Natural History, London (England), who discovered the similar mineral paratacamite. The mineral smithite is also named after him. Atacamite Group. 3 Quantum spin liquids: general definitions and properties... "Resonating valence-bond" (quantum spin liquid) states Idea: the best state for two spin-1/2 spins is a valence bond (a spin singlet):... Two-dimensional Kagome lattice: Herbertsmithite and Volborthite ZnCu3(OH)6Cl2 and Cu3V2O7(OH)2 2H2O.

A New State Of Matter: Quantum Spin Liquids Explained.

Quantum spin liquids form a novel class of matter where, despite the existence of strong exchange interactions, spins do not order down to the lowest measured temperature. Typically, these occur in lattices that act to frustrate the appearance of magnetism. In two dimensions, the classic example is the kagome lattice composed of corner sharing triangles.. A liquid-like state called a quantum spin liquid (QSL). The herbertsmithite ZnCu 3 (OH) 6 Cl 2 has been ex posed as a S = 1 / 2 kagome antiferromagnet, and recent ex. It has been suggested that the nearest-neighbor antiferromagnetic Heisenberg model on the Kagome lattice may be a good starting point for understanding the spin-liquid behavior discovered in herbertsmithite. In this work, we investigate possible quantum spin liquid phases in the presence of spin-rotation symmetry-breaking perturbations such as Dzyaloshinskii-Moriya and Ising interactions, as.

Symmetry Reduction in the Quantum Kagome Antiferromagnet Herbertsmithite.

Kitaev Spin Liquid Maria Hermanns, Stockholm University Nordita Tim Eschmann... Quantum spin liquids ‣ no magnetic order ‣ strongly fluctuating spins down to zero... Herbertsmithite ZnCu 3(OH) 6CL 2 Han et al., Nature (2012) Towards quantum spin liquids - frustration.

Gapless triangular-lattice spin-liquid candidate in PrZnAl$_{11}$O$_{19}.

. The frustrated magnet (insulator) herbertsmithite ZnCu 3 (OH) 6 Cl 2 is one of the best candidates for identification as a material that hosts a quantum spin liquid (QSL), thereby determining the nature of its thermodynamic, relaxation, and transport properties. The insulating nature of ZnCu 3 (OH) 6 Cl 2 has been established: There is a 3.3 eV charge gap (see e.g., [1,2]). An exotic quantum spin liquid (QSL) is formed with such hypothetic particles as fermionic spinons carrying spin 1/2 and no charge. Here we calculate its thermodynamic and relaxation properties.... This demonstrates that the spin liquid of herbertsmithite is close to QCP and behaves like the HF liquid of YbRh 2 Si 2 in strong magnetic fields.

Heat Transport in Herbertsmithite: Can a Quantum Spin Liquid.

Quantum Spin Liquid Pathway With potential roles in quantum computation, high-temperature superconductivity and a range of exotic anyonic states, why quantum spin liquids (QSLs) attract interest is no great mystery. [31]... (OH)6FCl and previously studied herbertsmithite Cu3Zn(OH)6Cl2 and Zn-doped Barlowite Cu3Zn(OH)6FBr. "Looking into the.

Li doped kagome spin liquid compounds - The College of.

We report 17O NMR measurements in the S=1/2 Cu2+ kagome antiferromagnet Herbertsmithite ZnCu3(OH)6Cl2 down to 45mK in magnetic fields ranging from 2T to 12T. While Herbertsmithite displays a gapless spin-liquid behavior in zero field, we uncover an instability toward a spin-solid phase at sub-kelvin temperature induced by an applied magnetic field. The latter phase shows largely suppressed.

For Newly Discovered 'Quantum Spin Liquid', the Beauty Is in.

Since the proposal by Anderson of the resonating valence bond state, 1) the quantum spin-liquid (QSL) state possibly realized in certain \(S = 1/2\) frustrated magnets has attracted interest of researchers. 2) After a long experimental quest, several candidate materials were recently reported in geometrically frustrated magnets, including both the triangular-lattice and the kagome-lattice. Called a Dirac spin liquid, is special, and is a candidate ground state for several sim-ple models as well as several materials (such as Herbertsmithite and Ba 8CoNb 6O 24). A Dirac spin liquid is described in terms of spin-half fermions with a massless Dirac dispersion, coupled to an emergent photon eld. This gauge theory is just like the. Quantum spin liquid candidate becomes a superconductor under pressure. According to the researchers, who present their results in Science, such defects may in fact prove crucial to the low-temperature magnetic properties of all quantum spin systems that lack magnetic order.Indeed, there are now only a few QSL candidates in which a spin gap has not been proven beyond any doubt, they explain.

Quantum Spin-Liquid Behavior in the Spin-1/2 Random-Bond Heisenberg.

When the randomness exceeds a critical value, the ground state of the model exhibits a transition within the non-magnetic state into the randomness-relevant gapless spin-liquid state. Implications to the S=1/2 kagome-lattice antiferromagnet herbertsmithite is discussed. Quantum spin liquid (QSL) represents a new state of matter characterized by long-range entanglement, beyond the conventional symmetry-breaking paradigm [1]. Realizing QSL in real-world materials has been a long-sought goal for decades [2-4]. The most promising candidate so far is herbertsmithite Cu 3Zn(OH) 6Cl 2, which realizes the S = 1/2. The conditions for a quantum spin liquid to arise are often found in nature, like in the magnetic layers of copper ions of the mineral Herbertsmithite. But synthetically creating this state of.

(PDF) Quantum Spin Liquid Pathway | George Rajna - A.

Abstract: Quantum spin liquids form a novel class of matter where, despite the existence of strong exchange interactions, spins do not order down to the lowest measured temperature. Typically, these occur in lattices that act to frustrate the appearance of magnetism. In two dimensions, the classic example is the kagome lattice composed of corner sharing. The conditions required for a quantum spin liquid to form are often found in nature. The most famous example is the copper-based mineral Herbertsmithite, for which there is significant evidence to. When the randomness exceeds a critical value, the ground state of the model exhibits a transition within the non-magnetic state into the randomness-relevant gapless spin-liquid state. Implications to the S=1/2 kagome-lattice antiferromagnet herbertsmithite is discussed.

Fractionalized excitations in the spin-liquid state of a.

"The structural simplicity of Herbertsmithite is valuable if we are to put the quantum spin liquid to use—as proposed for information processing, for example," he says. "Complex chemistry usually. The conditions required for a quantum spin liquid to form are often found in nature. The most famous example is the copper-based mineral Herbertsmithite, for which there is significant evidence to.

Evidence for a gapped spin-liquid ground state in a kagome... - AAAS.

Among the inorganic spin-liquid candidates, the rhombohedral herbertsmithite ZnCu 3 (OH) 6 Cl 2 scored highest in popularity. As depicted in figure 2, the copper ions form an almost perfect kagome lattice [], i.e. corner sharing triangles in the plane with strong antiferromagnetic superexchange J of approximately 200 K.

MIT demonstrates new magnetic state with quantum spin liquids.

The material in question is an example of an exotic phase of matter known as a quantum spin liquid,... Researchers in 2012 found a naturally occurring example in the mineral herbertsmithite.

Perfect Kagomé lattices in YCu3(OH)6Cl3: a new candidate for the.

We report a direct measurement of the low-frequency optical conductivity of large-area single-crystal herbertsmithite, a promising spin-liquid candidate material, by means of terahertz time-domain spectroscopy. In the spectral range below 1.4 THz, we observe a contribution to the real part of the in-plane conductivity ${\\ensuremath{\\sigma}}_{ab}(\\ensuremath{\\omega})$ from the spin degree.


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